Engineering Three Dimensional Moiré Flat Bands

Nano Letters 21,18, 7519 - 7526 (2021)

Engineering Three Dimensional Moiré Flat Bands

Lede Xian, Ammon Fischer, Martin Claassen, Jin Zhang, Angel Rubio, Dante M. Kennes

Twisting two adjacent layers of van der Waals materials with respect to each other can lead to flat two-dimensional electronic bands which enables a wealth of physical phenomena. Here, we generalize this concept of so-called moiré flat bands to engineer flat bands in all three spatial dimensions controlled by the twist angle. The basic concept is to stack the material such that the large spatial moiréinterference patterns are spatially shifted from one twisted layer to the next. We exemplify the general concept by considering graphitic systems, boron nitride, and WSe2, but the approach is applicable to any two-dimensional van der Waals material. For hexagonal boron nitride, we develop an ab initio fitted tight binding model that captures the corresponding three-dimensional low-energy electronic structure. We outline that interesting three-dimensional correlated phases of matter can be induced and controlled following this route, including quantum magnets and unconventional superconducting states.

Additional Information

Preprint - 6.35 MB

Related Projects

Related Research Areas